Carbon-supported Single-atom Metal Materials for Robust Li/Na/K Batteries: A Mini Review

Qiongguang Li; Menglei Yuan; Yaqin Wang; Meng Yao; Yanhong Wang; Ziyi Zhong; Fabing Su

doi:10.1016/j.mtsust.2023.100355

Carbon-supported Single-atom Metal Materials for Robust Li/Na/K Batteries: A Mini Review

Qiongguang Li^*, Menglei Yuan, Yaqin Wang, Meng Yao, Yanhong Wang, Ziyi Zhong, Fabing Su^*

^*Corresponding author for this work

Chemical Engineering

Research output: Contribution to journal › Article › peer-review

5 Scopus citations

Abstract

Alkali ion batteries have attracted broad attention because of their high power and energy density. However, there is an urgency to explore novel electrode materials with higher capacity and longer cycle life to meet the ever-increasing requirements. Due to their unique electronic structure and coordination environment, carbon-supported single-atom metal (CSAM) materials are promising to enhance the anode capacity and prolong its lifespan, but the development is still in its infancy stage. In this mini-review, we first summarize the application of CSAM materials in alkali ion batteries from theoretical predictions to experimental investigations. Then the work mechanisms of CSAM materials in alkali ion batteries are discussed, and their disadvantages, such as low mass loading, low activity and metal atom migration, are reviewed. Finally, we discuss the solution strategies to address these issues. This mini-review will guide the structural design of CSAM materials and accelerate the future application in alkali ion batteries.

Original language	English
Journal	Materials Today Sustainability
DOIs	https://doi.org/10.1016/j.mtsust.2023.100355
State	E-pub ahead of print - 10 Feb 2023

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title = "Carbon-supported Single-atom Metal Materials for Robust Li/Na/K Batteries: A Mini Review",

abstract = "Alkali ion batteries have attracted broad attention because of their high power and energy density. However, there is an urgency to explore novel electrode materials with higher capacity and longer cycle life to meet the ever-increasing requirements. Due to their unique electronic structure and coordination environment, carbon-supported single-atom metal (CSAM) materials are promising to enhance the anode capacity and prolong its lifespan, but the development is still in its infancy stage. In this mini-review, we first summarize the application of CSAM materials in alkali ion batteries from theoretical predictions to experimental investigations. Then the work mechanisms of CSAM materials in alkali ion batteries are discussed, and their disadvantages, such as low mass loading, low activity and metal atom migration, are reviewed. Finally, we discuss the solution strategies to address these issues. This mini-review will guide the structural design of CSAM materials and accelerate the future application in alkali ion batteries.",

author = "Qiongguang Li and Menglei Yuan and Yaqin Wang and Meng Yao and Yanhong Wang and Ziyi Zhong and Fabing Su",

year = "2023",

month = feb,

day = "10",

doi = "10.1016/j.mtsust.2023.100355",

language = "英语",

journal = "Materials Today Sustainability",

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TY - JOUR

T1 - Carbon-supported Single-atom Metal Materials for Robust Li/Na/K Batteries: A Mini Review

AU - Li, Qiongguang

AU - Yuan, Menglei

AU - Wang, Yaqin

AU - Yao, Meng

AU - Wang, Yanhong

AU - Zhong, Ziyi

AU - Su, Fabing

PY - 2023/2/10

Y1 - 2023/2/10

N2 - Alkali ion batteries have attracted broad attention because of their high power and energy density. However, there is an urgency to explore novel electrode materials with higher capacity and longer cycle life to meet the ever-increasing requirements. Due to their unique electronic structure and coordination environment, carbon-supported single-atom metal (CSAM) materials are promising to enhance the anode capacity and prolong its lifespan, but the development is still in its infancy stage. In this mini-review, we first summarize the application of CSAM materials in alkali ion batteries from theoretical predictions to experimental investigations. Then the work mechanisms of CSAM materials in alkali ion batteries are discussed, and their disadvantages, such as low mass loading, low activity and metal atom migration, are reviewed. Finally, we discuss the solution strategies to address these issues. This mini-review will guide the structural design of CSAM materials and accelerate the future application in alkali ion batteries.

AB - Alkali ion batteries have attracted broad attention because of their high power and energy density. However, there is an urgency to explore novel electrode materials with higher capacity and longer cycle life to meet the ever-increasing requirements. Due to their unique electronic structure and coordination environment, carbon-supported single-atom metal (CSAM) materials are promising to enhance the anode capacity and prolong its lifespan, but the development is still in its infancy stage. In this mini-review, we first summarize the application of CSAM materials in alkali ion batteries from theoretical predictions to experimental investigations. Then the work mechanisms of CSAM materials in alkali ion batteries are discussed, and their disadvantages, such as low mass loading, low activity and metal atom migration, are reviewed. Finally, we discuss the solution strategies to address these issues. This mini-review will guide the structural design of CSAM materials and accelerate the future application in alkali ion batteries.

U2 - 10.1016/j.mtsust.2023.100355

DO - 10.1016/j.mtsust.2023.100355

M3 - 文章

SN - 2589-2347

JO - Materials Today Sustainability

JF - Materials Today Sustainability

ER -

Carbon-supported Single-atom Metal Materials for Robust Li/Na/K Batteries: A Mini Review

Abstract

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