Membrane reactor design for thermally balanced hydrogen production

Stas A. Simakov; Moshe Sheintuch

Membrane reactor design for thermally balanced hydrogen production

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Abstract

Hydrogen production by steam reforming of methane or methanol in a catalytic fixed bed membrane reactor was investigated. Hydrogen separation by a permselective inorganic membrane, e.g., Pd, shifted the equilibrium of the steam reforming reaction. The endothermicity of the steam reforming was compensated by the combustion of methane or methanol. Two alternative designs for the thermal coupling of endothermic steam reforming and exothermic oxidation were compared. Since thermal fronts are formed, axial dispersion cannot be ignored. The thermally balanced reactor might be operated without heating. The reactor was designed to provide high purity hydrogen feed for fuel cells. Comparison with other approaches, like millisecond combustion, were discussed. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 1/04/2005).

Original language	English
Title of host publication	05AIChE
Subtitle of host publication	2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings
Publisher	American Institute of Chemical Engineers
ISBN (Print)	0816909962, 9780816909964
State	Published - 2005
Externally published	Yes
Event	05AIChE: 2005 AIChE Annual Meeting and Fall Showcase - Cincinnati, OH, United States Duration: 30 Oct 2005 → 4 Nov 2005

Publication series

Name	AIChE Annual Meeting Conference Proceedings
Volume	2005

Conference

Conference	05AIChE: 2005 AIChE Annual Meeting and Fall Showcase
Country/Territory	United States
City	Cincinnati, OH
Period	30/10/05 → 4/11/05

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This output contributes to the following UN Sustainable Development Goals (SDGs)

Cite this

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title = "Membrane reactor design for thermally balanced hydrogen production",

abstract = "Hydrogen production by steam reforming of methane or methanol in a catalytic fixed bed membrane reactor was investigated. Hydrogen separation by a permselective inorganic membrane, e.g., Pd, shifted the equilibrium of the steam reforming reaction. The endothermicity of the steam reforming was compensated by the combustion of methane or methanol. Two alternative designs for the thermal coupling of endothermic steam reforming and exothermic oxidation were compared. Since thermal fronts are formed, axial dispersion cannot be ignored. The thermally balanced reactor might be operated without heating. The reactor was designed to provide high purity hydrogen feed for fuel cells. Comparison with other approaches, like millisecond combustion, were discussed. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 1/04/2005).",

author = "Simakov, {Stas A.} and Moshe Sheintuch",

year = "2005",

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isbn = "0816909962",

series = "AIChE Annual Meeting Conference Proceedings",

publisher = "American Institute of Chemical Engineers",

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note = "05AIChE: 2005 AIChE Annual Meeting and Fall Showcase ; Conference date: 30-10-2005 Through 04-11-2005",

}

Simakov, SA & Sheintuch, M 2005, Membrane reactor design for thermally balanced hydrogen production. in 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings. AIChE Annual Meeting Conference Proceedings, vol. 2005, American Institute of Chemical Engineers, 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Cincinnati, OH, United States, 30/10/05.

Membrane reactor design for thermally balanced hydrogen production. / Simakov, Stas A.; Sheintuch, Moshe.
05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings. American Institute of Chemical Engineers, 2005. (AIChE Annual Meeting Conference Proceedings; Vol. 2005).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Membrane reactor design for thermally balanced hydrogen production

AU - Simakov, Stas A.

AU - Sheintuch, Moshe

PY - 2005

Y1 - 2005

N2 - Hydrogen production by steam reforming of methane or methanol in a catalytic fixed bed membrane reactor was investigated. Hydrogen separation by a permselective inorganic membrane, e.g., Pd, shifted the equilibrium of the steam reforming reaction. The endothermicity of the steam reforming was compensated by the combustion of methane or methanol. Two alternative designs for the thermal coupling of endothermic steam reforming and exothermic oxidation were compared. Since thermal fronts are formed, axial dispersion cannot be ignored. The thermally balanced reactor might be operated without heating. The reactor was designed to provide high purity hydrogen feed for fuel cells. Comparison with other approaches, like millisecond combustion, were discussed. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 1/04/2005).

AB - Hydrogen production by steam reforming of methane or methanol in a catalytic fixed bed membrane reactor was investigated. Hydrogen separation by a permselective inorganic membrane, e.g., Pd, shifted the equilibrium of the steam reforming reaction. The endothermicity of the steam reforming was compensated by the combustion of methane or methanol. Two alternative designs for the thermal coupling of endothermic steam reforming and exothermic oxidation were compared. Since thermal fronts are formed, axial dispersion cannot be ignored. The thermally balanced reactor might be operated without heating. The reactor was designed to provide high purity hydrogen feed for fuel cells. Comparison with other approaches, like millisecond combustion, were discussed. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 1/04/2005).

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M3 - 会议稿件

AN - SCOPUS:33646728005

SN - 0816909962

SN - 9780816909964

T3 - AIChE Annual Meeting Conference Proceedings

BT - 05AIChE

PB - American Institute of Chemical Engineers

T2 - 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase

Y2 - 30 October 2005 through 4 November 2005

ER -

Membrane reactor design for thermally balanced hydrogen production

Abstract

Publication series

Conference

UN SDGs

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