Bismuth and Metal-Doped Bismuth Nanoparticles Produced by Laser Ablation for Electrochemical Glucose Sensing

Weiran Zheng; Yong Li; Lawrence Yoon Suk Lee

doi:10.1016/j.snb.2021.131334

Bismuth and Metal-Doped Bismuth Nanoparticles Produced by Laser Ablation for Electrochemical Glucose Sensing

Weiran Zheng, Yong Li, Lawrence Yoon Suk Lee^*

^*Corresponding author for this work

Chemistry

Research output: Contribution to journal › Article › peer-review

11 Scopus citations

Abstract

Materials based on transition metals, such as Cu, Co, and Ni, have been intensively used as electrocatalysts for non-enzymatic electrochemical glucose sensing. However, the current trend of wearable/in vivo continuous glucose sensing has raised the need for non/low-toxic candidates. Herein, we demonstrate that the overlooked low-toxic bismuth (Bi)-based nanomaterials are suitable choices. Using a laser-ablation method, surfactant-free Bi nanoparticles (NPs) and transition metal (Ni and Co)-doped Bi NPs are obtained, achieving amperometric sensitivity values of 127, 677, and 2326 µA mM−1 cm−2, respectively. Low detection limits of 1 and 4 µM, as well as an extensive linear range of 0.001–3.5 mM, are recorded using Ni- and Co-doped Bi NPs, respectively. With competitive performance and high selectivity towards glucose sensing in both standard and serum samples, Bi-based nanomaterials are proven effective and promising candidates for future glucose sensor design beyond transition metal elements.

Original language	English
Journal	Sensors and Actuators B: Chemical
DOIs	https://doi.org/10.1016/j.snb.2021.131334
State	Published - 15 Apr 2022

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title = "Bismuth and Metal-Doped Bismuth Nanoparticles Produced by Laser Ablation for Electrochemical Glucose Sensing",

abstract = "Materials based on transition metals, such as Cu, Co, and Ni, have been intensively used as electrocatalysts for non-enzymatic electrochemical glucose sensing. However, the current trend of wearable/in vivo continuous glucose sensing has raised the need for non/low-toxic candidates. Herein, we demonstrate that the overlooked low-toxic bismuth (Bi)-based nanomaterials are suitable choices. Using a laser-ablation method, surfactant-free Bi nanoparticles (NPs) and transition metal (Ni and Co)-doped Bi NPs are obtained, achieving amperometric sensitivity values of 127, 677, and 2326 µA mM−1 cm−2, respectively. Low detection limits of 1 and 4 µM, as well as an extensive linear range of 0.001–3.5 mM, are recorded using Ni- and Co-doped Bi NPs, respectively. With competitive performance and high selectivity towards glucose sensing in both standard and serum samples, Bi-based nanomaterials are proven effective and promising candidates for future glucose sensor design beyond transition metal elements.",

author = "Weiran Zheng and Yong Li and Lee, {Lawrence Yoon Suk}",

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T1 - Bismuth and Metal-Doped Bismuth Nanoparticles Produced by Laser Ablation for Electrochemical Glucose Sensing

AU - Zheng, Weiran

AU - Li, Yong

AU - Lee, Lawrence Yoon Suk

PY - 2022/4/15

Y1 - 2022/4/15

N2 - Materials based on transition metals, such as Cu, Co, and Ni, have been intensively used as electrocatalysts for non-enzymatic electrochemical glucose sensing. However, the current trend of wearable/in vivo continuous glucose sensing has raised the need for non/low-toxic candidates. Herein, we demonstrate that the overlooked low-toxic bismuth (Bi)-based nanomaterials are suitable choices. Using a laser-ablation method, surfactant-free Bi nanoparticles (NPs) and transition metal (Ni and Co)-doped Bi NPs are obtained, achieving amperometric sensitivity values of 127, 677, and 2326 µA mM−1 cm−2, respectively. Low detection limits of 1 and 4 µM, as well as an extensive linear range of 0.001–3.5 mM, are recorded using Ni- and Co-doped Bi NPs, respectively. With competitive performance and high selectivity towards glucose sensing in both standard and serum samples, Bi-based nanomaterials are proven effective and promising candidates for future glucose sensor design beyond transition metal elements.

AB - Materials based on transition metals, such as Cu, Co, and Ni, have been intensively used as electrocatalysts for non-enzymatic electrochemical glucose sensing. However, the current trend of wearable/in vivo continuous glucose sensing has raised the need for non/low-toxic candidates. Herein, we demonstrate that the overlooked low-toxic bismuth (Bi)-based nanomaterials are suitable choices. Using a laser-ablation method, surfactant-free Bi nanoparticles (NPs) and transition metal (Ni and Co)-doped Bi NPs are obtained, achieving amperometric sensitivity values of 127, 677, and 2326 µA mM−1 cm−2, respectively. Low detection limits of 1 and 4 µM, as well as an extensive linear range of 0.001–3.5 mM, are recorded using Ni- and Co-doped Bi NPs, respectively. With competitive performance and high selectivity towards glucose sensing in both standard and serum samples, Bi-based nanomaterials are proven effective and promising candidates for future glucose sensor design beyond transition metal elements.

U2 - 10.1016/j.snb.2021.131334

DO - 10.1016/j.snb.2021.131334

M3 - 文章

SN - 0925-4005

JO - Sensors and Actuators B: Chemical

JF - Sensors and Actuators B: Chemical

ER -

Bismuth and Metal-Doped Bismuth Nanoparticles Produced by Laser Ablation for Electrochemical Glucose Sensing

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